Multi-Media Files Derived From Research (under development)

Professor Radhakrishna Sureshkumar, Washington University in Saint Louis

Biomolecular Dynamics

1.      Brownian Dynamics Simulation (BDS) of Wormlike DNA Molecules in Extensional Flow (3.5 MB) This movie illustrates the influence of extension rate on the dynamics of two molecules with identical initial conditions. The symbol “Wi” denotes the ratio of the characteristic time scales associated with chain relaxation and the flow. For Wi =100, the chain extends from a coiled to fully extended state fairly rapidly. In comparison, for Wi = 10, the configuration landscape is much more complex. In the latter case, the chain assumes different configurational states, i.e., fold, kink, dumbbell, half-dumbbell etc., before reaching a state with nearly full extension. 

2.      BDS of wormlike DNA Molecules in Acoustic Streaming Flow (6.2 MB) The movement of the red dot illustrates the motion of the center of mass of the molecule along the streamline. The configurations of three molecules from an ensemble of 2000 are shown inside. The flow is generated by acoustic wave propagation through the fluid.

3.      Breaking of a DNA molecule (modeled as a bead-rod or Kramers chain) in uniaxial extensional flow (3 MB)

Turbulent Drag Reduction by Polymeric Additives

4.      Contours of large positive (blue) and negative (red) streamwise vorticity and large molecular extension (yellow) in turbulent channel flow of a dilute polymer solution. Polymeric additives are used to reduce turbulent friction (by up to 70%) in fluid transportation lines (e.g. transatlantic oil transportation). Chain extension, especially around the vortices, enhances the resistance of the fluid to extensional deformation. This results in the stabilization of the streamwise vortices. Since a large amount of turbulent stress (Reynolds stress) is produced during the breakup of these vortices, their stabilization results in flow with reduced friction losses.

Elastic Flow Instability in Creeping Flow

5.      Nonlinear Evolution of Flow Instability in Creeping Flow of a Viscoelastic Polymer Solution (1 MB) Elastic normal stresses created by flow-induced stretching of polymer molecules can trigger instabilities in viscoelastic flows even when inertial forces are much smaller than viscous ones (i.e., creeping flow limit realized when the Reynolds number is much smaller than unity). This movie illustrates the nonlinear evolution of elastic instability in flow through a channel with sinusoidal walls (only a part of the bottom portion of the channel is shown; the flow is from left to right). Small perturbations in polymeric stress are “convected” by velocity gradients. This results in a new flow state with significantly larger chain extension at the contraction region.

6.      Streamlines (left) and Molecular Extension (right) in Flow between Eccentric Cylinders Gradient of elastic normal stress in a curvilinear flow is a harbinger of flow instability. 

Nonlinear Dynamics and Pattern Formation in Curvilinear Flows of Dilute Polymer Solutions

7.      Spiral Instability in Taylor-Couette Flow (1.4 MB) Polymeric additives can qualitatively alter flow transitions in Newtonian liquids. In the absence of viscoelastic polymer additives, centrifugal instability in Taylor-Couette flow (flow between independently rotating concentric cylinders) causes the development of stationary and axisymmetric vortices (Taylor vortices). Elastic forces caused by polymeric additives result in the formation of time-periodic and non-axisymmetric flow patterns such as spirals and ribbons (super-position of two spirals traveling in opposite directions). The movie illustrates the spiral pattern and its eventual transition to a ribbon-like structure as captured by direct numerical simulations. Higher order transitions, leading to phenomenon such as elastic turbulence, are under investigation.

Thermoelastic Instability

8.      Traveling Waves in Non-Isothermal  Flow

Digital Particle Imaging Velocimetry (DPIV)

9.      Tracking Elastic Flow Instabilities

10.  Effect of Surfactants on Mixing 

Morphological Transition in Interfacial Nanostructures

11.  Electropolymerized Coatings

12.  Effect of Surface Reaction Rate